Publication
Title
Spectral field mapping in plasmonic nanostructures with nanometer resolution
Author
Abstract
Plasmonic nanostructures and -devices are rapidly transforming light manipulation technology by allowing to modify and enhance optical fields on sub-wavelength scales. Advances in this field rely heavily on the development of new characterization methods for the fundamental nanoscale interactions. However, the direct and quantitative mapping of transient electric and magnetic fields characterizing the plasmonic coupling has been proven elusive to date. Here we demonstrate how to directly measure the inelastic momentum transfer of surface plasmon modes via the energy-loss filtered deflection of a focused electron beam in a transmission electron microscope. By scanning the beam over the sample we obtain a spatially and spectrally resolved deflection map and we further show how this deflection is related quantitatively to the spectral component of the induced electric and magnetic fields pertaining to the mode. In some regards this technique is an extension to the established differential phase contrast into the dynamic regime.
Language
English
Source (journal)
Nature communications
Publication
2018
ISSN
2041-1723
DOI
10.1038/S41467-018-06572-9
Volume/pages
9 (2018) , 6 p.
Article Reference
4207
ISI
000447074200005
Pubmed ID
30310063
Medium
E-only publicatie
Full text (Publisher's DOI)
Full text (open access)
UAntwerpen
Faculty/Department
Research group
Project info
ATOM: Advanced Holographic Tomographies for Nanoscale Materials: Revealing Electromagnetic and Deformation Fields, Chemical Composition and Quantum States at Atomic Resolution
Publication type
Subject
Affiliation
Publications with a UAntwerp address
External links
Web of Science
Record
Identifier
Creation 29.10.2018
Last edited 09.10.2023
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