Publication
Title
Controlling the interfacial conductance in in 90 degrees off-axis sputter deposition
Author
Abstract
We report on the fabrication of conducting interfaces between LaAlO3 and SrTiO3 by 90 degrees off-axis sputtering in an Ar atmosphere. At a growth pressure of 0.04 mbar the interface is metallic, with a carrier density of the order of 1 x 10(13) cm(-2) at 3 K. By increasing the growth pressure, we observe an increase of the out-of-plane lattice constants of the LaAlO3 films while the in-plane lattice constants do not change. Also, the low-temperature sheet resistance increases with increasing growth pressure, leading to an insulating interface when the growth pressure reaches 0.10 mbar. We attribute the structural variations to an increase of the La/Al ratio, which also explains the transition from metallic behavior to insulating behavior of the interfaces. Our research shows that the control which is furnished by the Ar pressure makes sputtering as versatile a process as pulsed laser deposition, and emphasizes the key role of the cation stoichiometry of LaAlO3 in the formation of the conducting interface.
Language
English
Source (journal)
Physical review materials / American Physical Society. - College Park, Md, 2017, currens
Publication
College Park, Md : American Physical Society , 2019
ISSN
2475-9953 [online]
DOI
10.1103/PHYSREVMATERIALS.3.034002
Volume/pages
3 :3 (2019) , 4 p.
Article Reference
034002
ISI
000461077100002
Medium
E-only publicatie
Full text (Publisher's DOI)
UAntwerpen
Faculty/Department
Research group
Project info
SOLARPAINT: Understanding the durability of light sensitive materials: transferring insights between solar cell physics and the chemistry of paintings.
Publication type
Subject
Affiliation
Publications with a UAntwerp address
External links
Web of Science
Record
Identifier
Creation 04.04.2019
Last edited 02.10.2024
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