|
Title
|
|
|
|
Spectroscopic coincidence experiments in transmission electron microscopy
|
|
|
Author
|
|
|
|
|
|
|
Abstract
|
|
|
|
| We demonstrate the feasibility of coincidence measurements on a conventional transmission electron microscope, revealing the temporal correlation between electron energy loss spectroscopy (EELS) and energy dispersive X-ray (EDX) spectroscopy events. We make use of a delay line detector with ps-range time resolution attached to a modified EELS spectrometer. We demonstrate that coincidence between both events, related to the excitation and deexcitation of atoms in a crystal, provides added information not present in the individual EELS or EDX spectra. In particular, the method provides EELS with a significantly suppressed or even removed background, overcoming the many difficulties with conventional parametric background fitting as it uses no assumptions on the shape of the background, requires no user input and does not suffer from counting noise originating from the background signal. This is highly attractive, especially when low concentrations of elements need to be detected in a matrix of other elements. |
|
|
|
Language
|
|
|
|
English
|
|
|
Source (journal)
|
|
|
|
Applied physics letters / American Institute of Physics. - New York, N.Y., 1962, currens
|
|
|
Related dataset(s)
|
|
|
|
|
|
|
Publication
|
|
|
|
New York, N.Y.
:
American Institute of Physics
,
2019
|
|
|
ISSN
|
|
|
|
0003-6951
[print]
1077-3118
[online]
|
|
|
DOI
|
|
|
|
10.1063/1.5092945
|
|
|
Volume/pages
|
|
|
|
114
:14
(2019)
, 5 p.
|
|
|
Article Reference
|
|
|
|
143101
|
|
|
ISI
|
|
|
|
000464450200022
|
|
|
Medium
|
|
|
|
E-only publicatie
|
|
|
Full text (Publisher's DOI)
|
|
|
|
|
|
|
Full text (open access)
|
|
|
|
|
|
|
Full text (publisher's version - intranet only)
|
|
|
|
|
|