Publication
Title
Atmospheric depletion of mercury over Antarctica during glacial periods
Author
Abstract
Mercury is a globally dispersed toxic metal that affects even remote polar areas. During seasonal atmospheric mercury depletion events in polar areas, mercury is removed from the atmosphere1, 2 and subsequently deposited in the surface snows3. However, it is unknown whether these events, which have been documented for the past two decades, have occurred in the past. Here we show that over the past 670,000 years, atmospheric mercury deposition in surface snows was greater during the coldest climatic stages, coincident with the highest atmospheric dust loads. A probable explanation for this increased scavenging is that the oxidation of gaseous mercury by sea-salt-derived halogens occurred in the cold atmosphere. The oxidized mercury compounds were then transferred to the abundant mineral dust particles and deposited on the snowpack, leading to the depletion of gaseous mercury in the Antarctic atmosphere. We conclude that polar regions acted as a mercury sink during the coldest climatic stages, and that substantial polar deposition of atmospheric mercury is therefore not an exclusively recent phenomenon.
Language
English
Source (journal)
Nature geoscience
Publication
2009
Volume/pages
2:7(2009), p. 505-508
ISI
000270061600021
Full text (Publisher's DOI)
UAntwerpen
Faculty/Department
Research group
Publication type
Subject
Affiliation
Publications with a UAntwerp address
External links
Web of Science
Record
Identification
Creation 06.07.2009
Last edited 24.08.2017
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